To avoid catastrophic consequences of climate change, our current carbon-emitting energy infrastructure needs to be replaced with an energy system free from atmospheric carbon emissions. The enormous scale of this energy transition requires multiple energy sources to be developed, including carbon-free wind, solar, geothermal, and nuclear as well as fossil-fuel-based systems where the carbon dioxide from the waste stream is captured and stored securely in deep subsurface geologic formations, in a technology known as Carbon Capture and Storage, or CCS. Subsurface geologic formations are also likely to be used to provide short-term storage for energy-carrying fluids like hydrogen and natural gas, making the subsurface environment critical to the energy transition. In this talk, I will discuss practical computational approaches to analyze geological storage systems as well as economic and political issues associated with CCS. I will also briefly discuss basic climate change facts, as part of a proposed general curriculum for Environmental Literacy.